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Mesoporous Silica with Site-Isolated Amine and Phosphotungstic Acid Groups: A Solid Catalyst with Tunable Antagonistic Functions for One-Pot Tandem Reactions

Shiju, N. Raveendran, Alberts, Albert H., Khalid, Syed, Brown, David .R. and Rothenberg, Gadi (2011) Mesoporous Silica with Site-Isolated Amine and Phosphotungstic Acid Groups: A Solid Catalyst with Tunable Antagonistic Functions for One-Pot Tandem Reactions. Angewandte Chemie International Edition, 50 (41). pp. 9615-9619. ISSN 14337851

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Abstract

Coniuga et impera: A bifunctional solid catalyst is prepared by combining acid and base functions on mesoporous silica supports (see picture). The co-existence of these functions is shown by a two-step reaction sequence in one pot. Excellent product yields, which cannot be obtained by separated acid and base functions in one pot, show the validity of our concept.

Item Type: Article
Subjects: Q Science > Q Science (General)
Q Science > QD Chemistry
Schools: School of Applied Sciences
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Depositing User: Sara Taylor
Date Deposited: 13 Oct 2011 16:23
Last Modified: 13 Oct 2011 16:23
URI: http://eprints.hud.ac.uk/id/eprint/11715

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